Principles Of Nonlinear Optical Spectroscopy

Nonlinear optical interaction of laser fields with matter provide powerful spectroscopic tools for the understanding of microscopic interactions and dynamic processes. This volume provides a systematic account of a wide class of nonlinear spectroscopic techniques, in time domain and frequency domain, for researchers and graduate students in the field. Current active research areas such as ultrafast time-domain techniques, the interplay of phase coherence in the matter and the coherence properties of the radiation field, experiments involving phase-controlled pulse sequences, and cooperative effects in nanostructures are emphasized. Annotation copyright by Book News, Inc., Portland, OR

This book reflects the latest advances in nonlinear optics. Besides the simple, strict mathematical deduction, it also discusses the experimental verification and possible future applications, such as the all-optical switches. It consistently uses the practical unit system throughout. It employs simple physical images, such as "light waves" and "photons" to systematically explain the main principles of nonlinear optical effects. It uses the first-order nonlinear wave equation in frequency domain under the condition of “slowly varying amplitude approximation" and the classical model of the interaction between the light and electric dipole. At the same time, it also uses the rate equations based on the energy-level transition of particle systems excited by photons and the energy and momentum conservation principles to explain the nonlinear optical phenomenon. The book is intended for researchers, engineers and graduate students in the field of optics, optoelectronics, fiber communication, information technology and materials etc.

Introduction to Nonlinear Laser Spectroscopy focuses on the principles of nonlinear laser spectroscopy. This book discusses the experimental techniques of nonlinear optics and spectroscopy. Comprised of seven chapters, this book starts with an overview of the stimulated Raman effect and coherent anti-Stokes Raman spectroscopy, which can be used in a varied way to generate radiation in the ultraviolet and vacuum-ultraviolet areas. This text then explains the simplest quantum-mechanical system consisting of an isolated entity with energy eigenstates

A comprehensive treatment of nonlinear optics emphasizing physical concepts and the relationhip between theory and experiment. Systematically describes a number of sub-topics in the field. Up-to-date references and numerous illustrations will help both beginners and practitioners interested in gaining a more thorough understanding of the subject.

For a host of reasons, nonlinear optical spectroscopy is a valuable tool for biochemical applications where minimally invasive diagnostics is desired. Biochemical Applications of Nonlinear Optical Spectroscopy presents the latest technological advances and offers a perspective on future directions in this important field. Written by an international panel of experts, this volume begins with a comparison of nonlinear optical spectroscopy and x-ray crystallography. The text examines the use of multiphoton fluorescence to study chemical phenomena in the skin, the use of nonlinear optics to enhance traditional optical spectroscopy, and the multimodal approach, which incorporates several spectroscopic techniques in one instrument. Later chapters explore Raman microscopy, third-harmonic generation microscopy, and non-linear Raman microspectroscopy. The text explores the promise of beam shaping and the use of broadband laser pulse generated through continuum generation and an optical pulse shaper. Lastly, the book discusses the effects of spatial beam shaping on the generated nonlinear Raman signals in a tightly focused geometry and provides insight into the extension of nonlinear optical spectroscopy to the nanoscale through the use of plasmonic tip-enhanced arrangement. With novel experimental approaches to this technology expanding day-by-day, the book’s balanced coverage from a wide range of international contributors not only elucidates important achievements, but also outlines future directions in this dynamic and promising field.

Nonlinear optics has been a rapidly growing field in recent decades. It is based on the study of effects and phenomena related to the interaction of intense coherent light radiation with matter. Physics of Nonlinear Optics describes various major nonlinear optical effects, including physical principles, experimental techniques, up-to-date research achievements, and current or potential applications. This book features clear conceptual descriptions, concise formulations, and emphasizes both theoretical and experimental aspects of nonlinear optics. The readability of this book is particularly enhanced by a series of color photographs showing the spectacular appearances of various nonlinear optical effects. Both authors of this book are outstanding research scientists renowned in their professional areas. Their major research achievements in nonlinear optics include the pioneering studies of two-wave-coupled refractive-index change, Raman-enhanced self-focusing, optical-frequency Pockels effect, stimulated Kerr scattering, optical phase-conjugation via backward stimulated emission, and two-photon-absorption based optical limiting, stabilization and reshaping.

Principles of Laser Spectroscopy and Quantum Optics is an essential textbook for graduate students studying the interaction of optical fields with atoms. It also serves as an ideal reference text for researchers working in the fields of laser spectroscopy and quantum optics. The book provides a rigorous introduction to the prototypical problems of radiation fields interacting with two- and three-level atomic systems. It examines the interaction of radiation with both atomic vapors and condensed matter systems, the density matrix and the Bloch vector, and applications involving linear absorption and saturation spectroscopy. Other topics include hole burning, dark states, slow light, and coherent transient spectroscopy, as well as atom optics and atom interferometry. In the second half of the text, the authors consider applications in which the radiation field is quantized. Topics include spontaneous decay, optical pumping, sub-Doppler laser cooling, the Heisenberg equations of motion for atomic and field operators, and light scattering by atoms in both weak and strong external fields. The concluding chapter offers methods for creating entangled and spin-squeezed states of matter. Instructors can create a one-semester course based on this book by combining the introductory chapters with a selection of the more advanced material. A solutions manual is available to teachers. Rigorous introduction to the interaction of optical fields with atoms Applications include linear and nonlinear spectroscopy, dark states, and slow light Extensive chapter on atom optics and atom interferometry Conclusion explores entangled and spin-squeezed states of matter Solutions manual (available only to teachers)

Two-Dimensional Optical Spectroscopy discusses the principles and applications of newly emerging two-dimensional vibrational and optical spectroscopy techniques. It provides a detailed account of basic theory required for an understanding of two-dimensional vibrational and electronic spectroscopy. It also bridges the gap between the formal developm

X-ray experiments have been used widely in materials science, and conventional spectroscopy has been based on linear responses in light–matter interactions. Recent development of ultrafast light sources of tabletop lasers and X-ray free electron lasers reveals nonlinear optical phenomena in the X-ray region, and the measurement signals have been found to carry a further wealth of information on materials. This book overviews such nonlinear X-ray spectroscopy and its related issues for materials science. Each chapter is written by pioneers in the field and skillfully reviews the topics of nonlinear spectroscopy including X-ray multi-photon absorption and X-ray second harmonic generation. The chapters are divided depending on photon wavelength, ranging from extreme ultraviolet to (soft) X-ray. To facilitate readers’ comprehensive understanding, some of the chapters cover the conventional linear X-ray spectroscopy and basic principles of the non-linear responses. The book is mainly accessible as a primer for junior/senior- or graduate-level readers, and it also serves as a useful reference or guide even for established researchers in optical spectroscopy. The book offers readers opportunities to benefit from cutting-edge research in this new area of nonlinear X-ray spectroscopy.