High Power And Efficient Mid Infrared Emitting Quantum Cascade Lasers

Learn how the rapidly expanding area of mid-infrared and terahertz photonics has been revolutionized in this comprehensive overview. State-of-the-art practical applications are supported by real-life examples and expert guidance. Also featuring fundamental theory enabling you to improve performance of both existing and future devices.

The active region of conventional Quantum Cascade Lasers (QCLs) is composed of quantum wells and barriers of fixed alloy composition. As a consequence, they suffer severe carrier leakage from the upper laser level, as evidenced by low characteristic-temperature values for both the threshold current density and the slope efficiency, over a wide range of heatsink temperatures above room temperature. Here, we describe three methods by which the performance of these devices can be substantially increased. First, to suppress carrier leakage, the energy separation between the upper laser level and the next-higher energy state in the active region, E54 (or E43), needs to be increased; to this end, we propose 4.8μm-emitting, step-tapered active-region (STA) QCLs for nearly complete suppression of carrier leakage. Secondly, we introduce an 8-9μm-emitting STA-QCL design, which also employs a miniband-like carrier extraction scheme to ensures rapid depopulation of the lower laser level. We call the fast, carrier-extraction scheme resonant extraction (RE) since it involves resonant-(tunneling)-extraction not only from lower active-region levels but also from the lower laser level. When both the STA concept and miniband-like carrier extraction scheme are applied, in so-called STA-RE QCLs, it is shown that record-high internal differential efficiency hid values of ~ 86% can be achieved, by comparison to the prior state-of-the-art values of 57 to 67%. Furthermore, the fundamental upper limit for hid is shown be ~ 90%. With this improvement to internal differential efficiency, the wall-plug efficiency, hwp of mid-infrared-emitting QCLs should be ~34% higher than previously predicted, with hwp reaching values in excess of 40% for 4.6μm-emitting QCLs. Preliminary results from 5.0μm-emitting STA-RE QCLs are shown. Lastly, we show how single QCL emitters can be monolithically beam-combined to create High-Index-Contrast Photonic-Crystal (HC-PC) lasers as a means to coherently scale a QCL's output power while maintaining high beam quality, even under continuous-wave (CW) operating conditions. We present one such structure, which provided an output power of 5.5 W in a far-field beam pattern with lobewidths ~1.65 times the diffraction limit, and 82% energy contained in the central lobe. Methods to further improve on this result are also discussed.

The book describes the most advanced techniques for generating coherent light in the mid-infrared region of the spectrum. These techniques represent diverse areas of photonics and include heterojunction semiconductor lasers, quantum cascade lasers, tunable crystalline lasers, fiber lasers, Raman lasers, and optical parametric laser sources. Offering authoritative reviews by internationally recognized experts, the book provides a wealth of information on the essential principles and methods of the generation of coherent mid-infrared light and on some of its applications. The instructive nature of the book makes it an excellent text for physicists and practicing engineers who want to use mid-infrared laser sources in spectroscopy, medicine, remote sensing and other fields, and for researchers in various disciplines requiring a broad introduction to the subject.

Quantum cascade laser (QCL) performance continues to improve towards the requirements of applications such as infrared counter measures. However, key metrics, such as wall-plug efficiency (WPE), are still not fully met. DARPA's EMIL program continues to support progress in QCLs, and this report summarizes the Princeton team's work during Phase I of this program. Although the work systematically addressed all major facets of efficiency, the greatest advancements involved injection designs, which improved almost all efficiency components. Strain compensated QCLs with heterogeneous injectors produced low voltage defect. The active core consisted of interdigitated undoped and doped injectors followed by nominally identical optical transitions. The undoped injectors were designed with reduced voltage defect while the doped injector designs were more conventional. The measured average voltage defect was less than 79 meV. At 80 K, a 2.3 mm long, back facet high reflectance coated laser had an emission wavelength of 4.7 micrometers and output 2.3 W pulsed power with 19% peak WPE. Other QCLs emitting at 4.2 micrometers featured a low voltage defect and short injector with only four quantum wells. Devices with a voltage defect of 20 meV and a record voltage efficiency of 91% were demonstrated for pulsed operation at 180 K. Voltage efficiencies of greater than 80% were exhibited at room temperature. WPEs ranging from 21% at cryogenic temperatures to 5.3% at room temperature were achieved. Interface roughness effects were analyzed as in homogeneous broadening, explaining the temperature dependent QCL gain spectra and suggesting improved designs. Specifically, density-matrix theory revealed benefits from stronger coupling between injector and upper laser level that led to low-temperature pulsed QCLs nearing 50% WPE.

Mid-infrared (mid-IR) quantum cascade lasers (QCLs) have been commercially available for low power applications, however, while the desire for higher power devices is present, the efficiency and reliability are severe limitations. This work takes a multi-faceted approach to improving the reliability and efficiency of QCLs including: the identification and mitigation of failure mechanisms under high power continuous wave (CW) and quasi-continuous wave (QCW) operation, optical and thermal modeling of devices to further reduce active region heating, verification of these models using charge-coupled device (CCD) based thermoreflectance, and the introduction of interface roughness (IFR) engineered devices to reduce IFR scattering and leakage. Atom probe tomography (APT) is also employed to investigate the amount of aluminum and gallium incorporation in thin InAlAs barriers and InGaAs wells. It was found that thin layers with thicknesses less than 2 nm require an intentional aluminum or gallium overshoot in the gas phase during growth to grow the targeted compositions. This was verified when the overshoot in thin barriers resulted in the convergence of modeled and experimental emitting wavelengths. APT was also used to interrogate a few key interfaces within a 40 stage strain-compensated QCL emitting near 4.6 [mu]m. This interrogation yielded both in-plane and axial IFR parameters for barriers of high and low aluminum incorporation, and in turn high and low strain, respectively. It was found that the barrier with the highest aluminum target had a nearly 50% larger root mean square (RMS) roughness when compared to the shorter barriers. As the IFR scattering is proportional to the square of both the RMS roughness and in-plane correlation length, this finding has a significant impact on the IFR scattering and leakage. The variable IFR parameters, axial correlation length, graded interfaces, graded lattice constants, graded conduction band edge, and quaternary alloy disorder (AD) scattering have been incorporated into a scattering model. Results from this model suggest lower global lifetimes and significantly reduced transition efficiencies which results in lower IFR leakage, however, if electronic temperatures from software using non-equilibrium Green's function (NGEF) is incorporated, leakage currents remain high.

A state-of-the-art overview of this rapidly expanding field, featuring fundamental theory, practical applications, and real-life examples.

This thesis presents the first comprehensive analysis of quantum cascade laser nonlinear dynamics and includes the first observation of a temporal chaotic behavior in quantum cascade lasers. It also provides the first analysis of optical instabilities in the mid-infrared range. Mid-infrared quantum cascade lasers are unipolar semiconductor lasers, which have become widely used in applications such as gas spectroscopy, free-space communications or optical countermeasures. Applying external perturbations such as optical feedback or optical injection leads to a strong modification of the quantum cascade laser properties. Optical feedback impacts the static properties of mid-infrared Fabry–Perot and distributed feedback quantum cascade lasers, inducing power increase; threshold reduction; modification of the optical spectrum, which can become either single- or multimode; and enhanced beam quality in broad-area transverse multimode lasers. It also leads to a different dynamical behavior, and a quantum cascade laser subject to optical feedback can oscillate periodically or even become chaotic. A quantum cascade laser under external control could therefore be a source with enhanced properties for the usual mid-infrared applications, but could also address new applications such as tunable photonic oscillators, extreme events generators, chaotic Light Detection and Ranging (LIDAR), chaos-based secured communications or unpredictable countermeasures.

An important guide to the major techniques for generating coherent light in the mid-infrared region of the spectrum Laser-based Mid-infrared Sources and Applications gives a comprehensive overview of the existing methods for generating coherent light in the important yet difficult-to-reach mid-infrared region of the spectrum (2–20 μm) and their applications. The book describes major approaches for mid-infrared light generation including ion-doped solid-state lasers, fiber lasers, semiconductor lasers, and laser sources based on nonlinear optical frequency conversion, and reviews a range of applications: spectral recognition of molecules and trace gas sensing, biomedical and military applications, high-field physics and attoscience, and others. Every chapter starts with the fundamentals for a given technique that enables self-directed study, while extensive references help conduct deeper research. Laser-based Mid-infrared Sources and Applications provides up-to-date information on the state-of the art mid-infrared sources, discusses in detail the advancements made over the last two decades such as microresonators and interband cascade lasers, and explores novel approaches that are currently subjects of intense research such as supercontinuum and frequency combs generation. This important book: • Explains the fundamental principles and major techniques for coherent mid-infrared light generation • Discusses recent advancements and current cutting-edge research in the field • Highlights important biomedical, environmental, and military applications Written for researchers, academics, students, and engineers from different disciplines, the book helps navigate the rapidly expanding field of mid-infrared laser-based technologies.

Coherent power scaling of quantum cascade lasers (QCLs) for high-power, single-mode continuous-wave (CW) operation has proven to be quite a difficult task - while the device volume could be scaled for higher output power, many other factors such as beam quality and thermal resistance are negatively impacted if the device design is not carefully considered. The main objective of this work has been to develop methods for realizing high continuous-wave (CW) output power QCLs with high beam quality and minimal beam steering. One attractive approach for tackling this problem is the use of resonant leaky-wave-coupled antiguided phase-locked laser arrays. This dissertation focusses on two approaches to achieve high coherent power: 1) one alternate to the resonant leaky-wave-coupled antiguided phase-locked array concept, so called 'reverse-taper'laser; and 2) one combining grating-coupled surface-emitting lasers (GCSELs) with resonant leaky-wave-coupled antiguided phase-locked arrays, where each array element is coupled in both the lateral and longitudinal direction; thus, has a potential for multi-watt -CW surface-emitted output powers with good beam quality and narrow spectral linewidth. The novel geometry reverse-taper QCL device can scale the output power while maintaining good beam quality and beam stability - the tapered region scales the output power, while the emitting facet is located at the narrow-end taper section, which provides mode filtering by suppressing high-order spatial modes. A small degree of collimated-beam centroid movement (