High Performance Mid Infrared Emitting Quantum Cascade Lasers

The active region of conventional Quantum Cascade Lasers (QCLs) is composed of quantum wells and barriers of fixed alloy composition. As a consequence, they suffer severe carrier leakage from the upper laser level, as evidenced by low characteristic-temperature values for both the threshold current density and the slope efficiency, over a wide range of heatsink temperatures above room temperature. Here, we describe three methods by which the performance of these devices can be substantially increased. First, to suppress carrier leakage, the energy separation between the upper laser level and the next-higher energy state in the active region, E54 (or E43), needs to be increased; to this end, we propose 4.8μm-emitting, step-tapered active-region (STA) QCLs for nearly complete suppression of carrier leakage. Secondly, we introduce an 8-9μm-emitting STA-QCL design, which also employs a miniband-like carrier extraction scheme to ensures rapid depopulation of the lower laser level. We call the fast, carrier-extraction scheme resonant extraction (RE) since it involves resonant-(tunneling)-extraction not only from lower active-region levels but also from the lower laser level. When both the STA concept and miniband-like carrier extraction scheme are applied, in so-called STA-RE QCLs, it is shown that record-high internal differential efficiency hid values of ~ 86% can be achieved, by comparison to the prior state-of-the-art values of 57 to 67%. Furthermore, the fundamental upper limit for hid is shown be ~ 90%. With this improvement to internal differential efficiency, the wall-plug efficiency, hwp of mid-infrared-emitting QCLs should be ~34% higher than previously predicted, with hwp reaching values in excess of 40% for 4.6μm-emitting QCLs. Preliminary results from 5.0μm-emitting STA-RE QCLs are shown. Lastly, we show how single QCL emitters can be monolithically beam-combined to create High-Index-Contrast Photonic-Crystal (HC-PC) lasers as a means to coherently scale a QCL's output power while maintaining high beam quality, even under continuous-wave (CW) operating conditions. We present one such structure, which provided an output power of 5.5 W in a far-field beam pattern with lobewidths ~1.65 times the diffraction limit, and 82% energy contained in the central lobe. Methods to further improve on this result are also discussed.

Learn how the rapidly expanding area of mid-infrared and terahertz photonics has been revolutionized in this comprehensive overview. State-of-the-art practical applications are supported by real-life examples and expert guidance. Also featuring fundamental theory enabling you to improve performance of both existing and future devices.

A state-of-the-art overview of this rapidly expanding field, featuring fundamental theory, practical applications, and real-life examples.

This work describes the work performed by the author at the ETH Zurich, under the supervision of Prof. Jerome Faist on the optimization of high performance quantum cascade lasers (QCLs) in the Mid-IR spectral region. The main factors influencing laser performance have therefore been analyzed. In particular the optimization of the laser design in order to improve the electron tranport and the optical gain. In addition a detailed analysis of the fabrication process is performed and a novel process scheme is presented for buried heterostructure lasers.

This thesis presents the first comprehensive analysis of quantum cascade laser nonlinear dynamics and includes the first observation of a temporal chaotic behavior in quantum cascade lasers. It also provides the first analysis of optical instabilities in the mid-infrared range. Mid-infrared quantum cascade lasers are unipolar semiconductor lasers, which have become widely used in applications such as gas spectroscopy, free-space communications or optical countermeasures. Applying external perturbations such as optical feedback or optical injection leads to a strong modification of the quantum cascade laser properties. Optical feedback impacts the static properties of mid-infrared Fabry–Perot and distributed feedback quantum cascade lasers, inducing power increase; threshold reduction; modification of the optical spectrum, which can become either single- or multimode; and enhanced beam quality in broad-area transverse multimode lasers. It also leads to a different dynamical behavior, and a quantum cascade laser subject to optical feedback can oscillate periodically or even become chaotic. A quantum cascade laser under external control could therefore be a source with enhanced properties for the usual mid-infrared applications, but could also address new applications such as tunable photonic oscillators, extreme events generators, chaotic Light Detection and Ranging (LIDAR), chaos-based secured communications or unpredictable countermeasures.

The mid-infrared domain is a promising optical domain because it holds two transparency atmospheric windows, as well as the fingerprint of many chemical compounds. Quantum cascade lasers (QCLs) are one of the available sources in this domain and have already been proven useful for spectroscopic applications and free-space communications. This thesis demonstrates how to implement a private free-space communication relying on mid-infrared optical chaos and this requires an accurate cartography of non-linear phenomena in quantum cascade lasers. This private transmission is made possible by the chaos synchronization of two twin QCLs. Chaos in QCLs can be generated under optical injection or external optical feedback. Depending on the parameters of the optical feedback, QCLs can exhibit several non-linear phenomena in addition to chaos. Similarities exist between QCLs and laser diodes when the chaotic dropouts are synchronized with an external modulation, and this effect is known as the entrainment phenomenon. With a cross-polarization reinjection technique, QCLs can generate all-optical square-waves. Eventually, it is possible to trigger optical extreme events in QCLs with tilted optical feedback. All these experimental results allow a better understanding of the non-linear dynamics of QCLs and will extend the potential applications of this kind of semiconductor lasers.

When using conventional substrates, such as InP and GaAs, the materials constituting the superlattice (SL) core region of the quantum cascade laser (QCL) are constrained by strain-induced critical-thickness limitations. Metamorphic buffer layers (MBLs) can serve as "virtual substrates" with a designer-chosen surface lattice constant, thus expanding the compositional-design space for a variety of device structures, including short-wavelength QCLs. An optimized short-wavelength (3.4 [mu]m) single-phonon-resonant (SPR)+ miniband extraction QCL design, grown on an [InxGa1-xAs] MBL, is presented along with the optical and thermal device considerations in play. MBLs can be grown with a variety of graded regions such as linear composition grade from GaAs to [InxGa1-xAs] or by employing dislocation filters between Si substrate and InP. QCL and test superlattices' regrowth on these MBLs with the corresponding materials and device analysis, is presented in this work. In addition to the materials limitation for the design of QCL devices, the requirement to have the constituent layers (1-5 nm) to be precisely controlled in the various compositions and thicknesses, is a challenge. Interfacial grading in strained SLs is studied via atom probe tomography for SLs with various layer thicknesses and relative lattice strains. The tip reconstructions are analyzed by fitting the interfaces to diffusion profiles. Mechanisms possible for the observed interdiffusion profile, such as surface segregation and/or bulk diffusion, are discussed. With an understanding of the compositional gradient at the interfaces, together with optimized QCL designs and regrowth on the MBLs, short-wavelength QCLs with high performances can be achieved

This collection of authoritative reviews by leading experts provides a broad and instructive introduction to the most advanced techniques for generating coherent light in the mid-infrared region of the spectrum. With a wealth of up-to-date references – also available online.

Coherent power scaling of quantum cascade lasers (QCLs) for high-power, single-mode continuous-wave (CW) operation has proven to be quite a difficult task - while the device volume could be scaled for higher output power, many other factors such as beam quality and thermal resistance are negatively impacted if the device design is not carefully considered. The main objective of this work has been to develop methods for realizing high continuous-wave (CW) output power QCLs with high beam quality and minimal beam steering. One attractive approach for tackling this problem is the use of resonant leaky-wave-coupled antiguided phase-locked laser arrays. This dissertation focusses on two approaches to achieve high coherent power: 1) one alternate to the resonant leaky-wave-coupled antiguided phase-locked array concept, so called 'reverse-taper'laser; and 2) one combining grating-coupled surface-emitting lasers (GCSELs) with resonant leaky-wave-coupled antiguided phase-locked arrays, where each array element is coupled in both the lateral and longitudinal direction; thus, has a potential for multi-watt -CW surface-emitted output powers with good beam quality and narrow spectral linewidth. The novel geometry reverse-taper QCL device can scale the output power while maintaining good beam quality and beam stability - the tapered region scales the output power, while the emitting facet is located at the narrow-end taper section, which provides mode filtering by suppressing high-order spatial modes. A small degree of collimated-beam centroid movement (