Development Of Terahertz Systems Using Quantum Cascade Lasers And Photomixers

Quantum cascade lasers (QCLs) are attractive for high-resolution spectroscopy because they can provide high power and a narrow linewidth. They are particularly promising in the terahertz (THz) range since they can be used as local oscillators for heterodyne detection as well as transmitters for direct detection. However, THz QCL-based technologies are still under development and are limited by the lack of frequency tunability as well as the frequency and output power stability for free-running operation. In this dissertation, frequency tuning and linewidth of THz QCLs are studied in detail by using rotational spectroscopic features of molecular species. In molecular spectroscopy, the Doppler eff ect broadens the spectral lines of molecules in the gas phase at thermal equilibrium. Saturated absorption spectroscopy has been performed that allows for sub-Doppler resolution of the spectral features. One possible application is QCL frequency stabilization based on the Lamb dip. Since the tunability of the emission frequency is an essential requirement to use THz QCL for high-resolution spectroscopy, a new method has been developed that relies on near-infrared (NIR) optical excitation of the QCL rear-facet. A wide tuning range has been achieved by using this approach. The scheme is straightforward to implement, and the approach can be readily applied to a large class of THz QCLs. The frequency and output stability of the local oscillator has a direct impact on the performance and consistency of the heterodyne spectroscopy. A technique has been developed for a simultaneous stabilization of the frequency and output power by taking advantage of the frequency and power regulation by NIR excitation. The results presented in this thesis will enable the routine use of THz QCLs for spectroscopic applications in the near future.

In this work we concentrate our efforts on the generation of laser emission at low THz frequencies (3-1 THz range) employing the quantum cascade technology. Quantum cascade (QC) lasers are unipolar semiconductor lasers based on intersubband transitions in quantum wells that cover a large portion of the Mid and Far Infrared electromagnetic spectrum. Two main research lines have been followed: (i) the development of quantum cascade lasers based on population inversion between parabolic subbands and (ii) the development of low frequency QC lasers based on a three-dimensional electron confinement induced by an external magnetic field. (i) : Gain and laser action have been demonstrated in different systems at frequencies of 3.4 3.6 THz exploiting bound-to-bound and bound-to-continuum optical transition. A QC laser emitting at 3.6 THz and based on a vertical transition and resonant tunneling in a single quantum well has been demonstrated. To overcome the limitations in performance of such a system, an heterostructure laser based on a bound-to-continuum transition has been developed. The structure was the first one to operate above the technologically important temperature of liquid nitrogen. With a further development of the bound-to-continuum design that includes lower state lifetime reduction by optical phonon emission, laser action was successfully achieved at 115 K.A study of different waveguide mechanisms suitable for different THz frequencies has also been carried out. (ii) : THz quantum cascade lasers based on the in-plane confinement introduced by a strong magnetic field applied perpendiculary to the plane of the layers have been developed. A model system based on large single quantum wells (50-60 nm wide) has been exploited to study this gain mechanism. Such an approach led to the extension of the frequency range of operation of QC lasers, with the demonstration of laser action at 1.39 THz (220 mm) which is the lowest frequency observed to-date for this kind of.

The recent development of easy-to-use sources and detectors of terahertz radiation has enabled growth in applications of terahertz (Thz) imaging and sensing. This vastly adaptable technology offers great potential across a wide range of areas, and the Handbook of terahertz technology for imaging, sensing and communications explores the fundamental principles, important developments and key applications emerging in this exciting field. Part one provides an authoritative introduction to the fundamentals of terahertz technology for imaging, sensing and communications. The generation, detection and emission of waves are discussed alongside fundamental aspects of surface plasmon polaritons, terahertz near-field imaging and sensing, room temperature terahertz detectors and terahertz wireless communications. Part two goes on to discuss recent progress and such novel techniques in terahertz technology as terahertz bio-sensing, array imagers, and resonant field enhancement of terahertz waves. Fiber-coupled time-domain spectroscopy systems (THz-TDS), terahertz photomixer systems, terahertz nanotechnology, frequency metrology and semiconductor material development for terahertz applications are all reviewed. Finally, applications of terahertz technology are explored in part three, including applications in tomographic imaging and material spectroscopy, art conservation, and the aerospace, wood products, semiconductor and pharmaceutical industries. With its distinguished editor and international team of expert contributors, the Handbook of terahertz technology for imaging, sensing and communications is an authoritative guide to the field for laser engineers, manufacturers of sensing devices and imaging equipment, security companies, the military, professionals working in process monitoring, and academics interested in this field. Examines techniques for the generation and detection of terahertz waves Discusses material development for terahertz applications Explores applications in tomographic imaging, art conservation and the pharmaceutical and aerospace industries

The book presents information about Terahertz science, Terahertz photodetectors and Terahertz Lasers. A special emphasis is given to room temperature operation of long wavelength photodetectors based on novel quantum dots (Centered Defect Spherical Quantum Dots). Moreover, a complete analysis of systems based on Quantum Cascade structures to detect far infrared wavelengths is provided. Finally, the book presents Terahertz laser principles considering multi-color lasers in this range of wavelengths. Written as a background for graduate students in the Optics field.

This book covers the latest advances in the techniques employed to manage the THz radiation and its potential uses. It has been subdivided in three sections: THz Detectors, THz Sources, Systems and Applications. These three sections will allow the reader to be introduced in a logical way to the physics problems of sensing and generation of the terahertz radiation, the implementation of these devices into systems including other components and finally the exploitation of the equipment for real applications in some different field. All of the sections and chapters can be individually addressed in order to deepen the understanding of a single topic without the need to read the whole book. The THz Detectors section will address the latest developments in detection devices based on three different physical principles: photodetection, thermal power detection, rectification. The THz Sources section will describe three completely different generation methods, operating in three separate scales: quantum cascade lasers, free electron lasers and non-linear optical generation. The Systems and Applications section will take care of introducing many of the aspects needed to move from a device to an equipment perspective: control of terahertz radiation, its use in imaging or in spectroscopy, potential uses in security, and will address also safety issues. The text book is at a level appropriate to graduate level courses up to researchers in the field who require a reference book covering all aspects of terahertz technology.

The terahertz or the far-infrared frequency range of the electromagnetic spectrum (...) has historically been technologically underdeveloped despite having many potential applications, primarily due to lack of suitable sources of coherent radiation. Following on the remarkable development of mid-infrared (...) quantum-cascade lasers (QCLs) in the past decade, this thesis describes the development of electrically-pumped terahertz quantum-cascade lasers in GaAs/AlsGal_. As heterostructures that span a spectral range of 1.59 - 5.0 THz (...). A quantum-cascade laser (QCL) emits photons due to electronic intersubband transitions in the quantum-wells of a semiconductor heterostructure. The operation of terahertz QCLs at frequencies below the Reststrahlen band in the semiconductor (...), is significantly more challenging as compared to that of the mid-infrared QCLs. Firstly, due to small energy separation between the laser levels various intersubband scattering mechanisms are activated, which make it difficult to selectively depopulate the lower laser level. Additionally, as electrons gain enough kinetic energy in the upper laser level thermally activated longitudinal-optical (LO) phonon scattering reduces the level lifetime and makes it difficult to sustain population inversion at higher temperatures. Secondly, waveguide design for terahertz mode confinement is also more challenging due to higher free-carrier losses in the semiconducting doped regions at the terahertz frequencies. For successful designs reported in this work, the lower radiative state depopulation is achieved by a combination of resonant-tunneling and fast LO phonon scattering, which allow robust operation even at relatively high temperatures. An equally important enabling mechanism for these lasers is the development of metal-metal waveguides, which provide low waveguides losses, and strong mode confinement due to subwavelength mode localization in the vertical dimension. With these techniques some record performances for terahertz QCLs are demonstrated including the highest pulsed operating temperature of 169 K, the highest continuous-wave (cw) operating temperature of 117 K, and the highest optical power output (248 mW in pulsed and 138 mW in cw at 5 K) for any terahertz QCL. Towards the bigger goal of realizing a 1-THz solid-state laser to ultimately bridge the gap between electronic and optical sources of electromagnetic radiation, QCLs with a unique one-well injection scheme, which minimizes intersubband absorption losses that occur at longer wavelengths, are developed. Based on this scheme a QCL operating at 1.59 THz (A - 189 ym) is realized, which is amongst the lowest frequency solid-state lasers that operate without the assistance of a magnetic field. This thesis also reports on the development of distributed-feedback lasers in metal-metal waveguides to obtain single-mode operation, with greater output power and better beam quality. The subwavelength vertical dimension in these waveguides leads to a strongly coupled DFB action and a large reflection from the end-facets, and thus conventional coupled-mode theory is not directly applicable to the DFB design. A design technique with precise control of phase of reflection at the end-facets is developed with the aid of finite-element analysis, and with some additional unique design and fabrication methods, robust DFB operation has been obtained. Single-mode surface-emitting terahertz QCLs operating up to - 150 K are demonstrated, with different grating devices spanning a range of approximately 0.35 THz around v - 3 THz using the same gain medium. A single-lobed far-field radiation pattern, higher output power due to surface-emission, and a relatively small degradation in temperature performance compared to the Fabry-Perot ridge lasers makes these DFB lasers well suited for practical applications that are being targeted by the terahertz quantum-cascade lasers.

The terahertz (THz) spectral range is devoid of commercially feasible radiation sources, detectors, and components. In particular, THz sources are bulky, complex to operate, and cost-prohibitive - more suited for a research laboratory than a commercial setting. Developing compact and mass-producible sources in the 1 to 6 THz spectral range will open up new avenues for this technology to make a mainstream societal impact. The focus of this thesis is the development of compact, room-temperature terahertz sources based on quantum cascade lasers (QCL) and quantum well technology. QCLs are semiconductor lasers that operate with high power at mid-infrared (mid-IR) and THz frequencies. THz QCLs are the only mW-level average power sources with spectral coverage from 0.8 to 5 THz. However they only work at cryogenic temperatures because they cannot maintain population inversion across the lasing transition at elevated temperatures. Cryogenic cooling makes these sources cumbersome to operate and expensive to manufacture. Room-temperature operation significantly enhances their commercial appeal and a portion of this dissertation investigated the improvement in THz QCL temperature performance using GaAs-Al0.15Ga0.85As double-phonon resonant active region designs. These devices worked up to 173 K and were a substantial improvement compared to prior implementations of double-phonon resonant designs. Room-temperature THz sources that do not require population inversion across the lasing transition can be engineered by combining the field of nonlinear optics with intersubband transitions in quantum well structures. One method of creating inversionless THz lasing is based upon the principle of Raman gain in semiconductors and this thesis explores the design of an intersubband Raman laser (IRL) with GaAs-Al0.33Ga0.67As heterostructures. The primary focus of this dissertation is developing room-temperature, broadly-tunable, monolithic THz sources based on difference-frequency generation (DFG) in mid-IR QCLs. The source active region is quantum-engineered to provide lasing at mid-IR frequencies, [omega]1 and [omega]2, and simultaneously have giant second-order optical nonlinearity for THz generation at frequency [omega] [subscript THz]=[omega]1-[omega]2. This dissertation developed a Cherenkov emission scheme that produced devices with a narrow emission linewidth, 0.12 mW peak power and tuning from 1.55 to 5.7 THz - the largest tuning bandwidth compared to semiconductor technology of similar size and cost.

Learn how the rapidly expanding area of mid-infrared and terahertz photonics has been revolutionized in this comprehensive overview. State-of-the-art practical applications are supported by real-life examples and expert guidance. Also featuring fundamental theory enabling you to improve performance of both existing and future devices.